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11.
Shuyi Fu Wenrui Feng Ying Jia Tielong Deng Wenzhong Wang Guling Zhang Junli Fu 《International Journal of Hydrogen Energy》2021,46(21):11544-11555
ZnO/Cu2S nanotube arrays are fabricated firstly by a facile and capping-agent-free method, and the photo-electrochemical performance has been studied systematically. The results show that ZnO/Cu2S nanotube arrays achieve enhanced photo-electrochemical water splitting performance and the photocurrent densities of ZnO/Cu2S are 7.9 times than that of ZnO at 0 V versus Ag/AgCl. The performance of the ZnO/Cu2S nanotube arrays can be adjusted by changing the amount of Cu2S microcrystals. The results confirm that the enhanced photo-electrochemical performance of ZnO/Cu2S is due to the significantly improved visible light absorption, effective separation of photo-induced carriers due to the well band energy match and the formed p-n junction between ZnO and Cu2S. 相似文献
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Wei Lai Lihong Ge Huaming Li Yilin Deng Bin Xu Bo Ouyang Erjun Kan 《International Journal of Hydrogen Energy》2021,46(53):26861-26872
The electrochemical water splitting to produce H2 in high efficiency with earth-abundant-metal catalysts remains a challenge. Here, we describe a simple “cyclic voltammetry + ageing” protocol at room temperature to activate Ni electrode (AC-Ni/NF) for hydrogen evolution reaction (HER), by which Ni/Ni(OH)2 heterostructure is formed at the surface. In situ Raman spectroscopy reveals the gradual growth of Ni/Ni(OH)2 heterostructure during the first 30 min of the aging treatment and combined with polarization measurements, it suggests a positive relation between the Ni/Ni(OH)2 amount and HER performance of the electrode. The obtained AC-Ni/NF catalyst, with plentiful Ni–Ni(OH)2 interfaces, exhibits remarkable performance towards HER, with the low overpotential of only 30 mV at a H2-evolving current density of 10 mA/cm2 and 153 mV at 100 mA/cm2, as well as a small Tafel slope of 46.8 mV/dec in 1 M KOH electrolyte at ambient temperature. The excellent HER performance of the AC-Ni/NF could be maintained for at least 24 h without obvious decay. Ex situ experiments and in situ electrochemical-Raman spectroscopy along with density functional theory (DFT) calculations reveal that Ni/Ni(OH)2 heterostructure, although partially reduced, can still persist during HER catalysis and it is the Ni–Ni(OH)2 interface reducing the energy barrier of H1 adsorption thus promoting the HER performance. 相似文献
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以Ti6Al4V球形粉末为原料,利用激光选区熔化成形方法制备了Ti6Al4V合金试样,采用光学显微镜、扫描电镜及力学性能测试等手段,研究了退火工艺对Ti6Al4V合金室温力学性能及组织的影响规律。结果表明: SLM成形沉积态Ti6Al4V合金室温抗拉强度超过1200 MPa,而平均断后伸长率仅为4.0%;在650 ℃下进行真空退火处理,合金的抗拉强度仍保持在1200 MPa左右,规定塑性延伸强度Rp0.2高于1150 MPa,但试样的断后伸长率<10%;而在750及800 ℃下进行真空退火处理,合金试样的抗拉强度降至1100 MPa左右,规定塑性延伸强度高于1050 MPa,伸长率达到甚至超过10%,材料的综合强韧性得到明显提升。随着真空退火加热温度和保温时间的增加,SLM成形Ti6Al4V合金原始β晶界逐渐变模糊,晶粒趋向于等轴化。与此同时,快速冷却转变的α′针状马氏体未出现明显地粗化。 相似文献
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In this paper, permanent magnet synchronous motors (PMSMs) are investigated. According to the feature of PMSMs, a novel state equation of PMSMs is obtained by choosing suitable state variables. Based on the state equation, robust controllers are designed via interval matrix and PI control idea. In terms of bilinear matrix inequations, sufficient conditions for the existence of the robust controller are derived. In order to reduce the conservation and the dependence on parameter, the control inputs of PMSMs are divided into two parts, a feedforward control input and a feedback control input, and relevant sufficient conditions for the existence of the controller are obtained. Because of the suitable choice of state variables, the proposed control strategies can cope with the load uncertainty and have robustness for disturbance. Finally, simulations are carried out via Matlab/Simulink soft to verify the effectiveness of the proposed control strategies. The performance of the proposed control strategies are demonstrated by the simulation results. 相似文献
16.
Chuang Yu Yu Yang Ze-xiang Wu Ji-fang Jiang Rao-ping Liao Yong-feng Deng 《Geotextiles and Geomembranes》2021,49(2):413-419
Geosynthetic clay liners (GCLs), which have a very low permeability to water and a considerably high self-healing capacity, are widely used in liner systems of landfills. In this study, a series of experimental tests were carried out under complex conditions on typical commercial GCLs from China. In particular, the effects of pH values and lead ions (Pb2+) were tested in addition to other factors. The swelling properties of natural bentonite encapsulated between geotextile components in the GCLs were tested first. The swelling capacity was reduced rapidly at pH values < 3 and concentrations of Pb2+ >40 mM. Permeability tests on GCLs with different concentrations of lead ions were then performed by using the self-developed multi-link flexible wall permeameter, and data showed that increases in lead ion concentrations greatly improved the permeability. Finally, self-healing capacity tests were conducted on needle-punched GCLs under different levels of damage. Results showed that the GCLs have a good self-healing capacity with small diameter damage holes (2 mm, close to three times the original aperture), but with a damage aperture larger than 15% of the sample area, the self-healing capacity could not prevent leakage; hence, in certain situations it will be necessary to repair the damage to meet the anti-seepage requirement. 相似文献
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黄冈大别山世界地质公园拥有4大类12亚类53处地质遗迹资源,为中国自太古代以来的中央造山带形成演化的天然实验室,大别山地区旅游资源丰富。游客量和旅游收入逐年稳步增加,但公园旅游客源地空间的集中程度高,以湖北省武汉市游客为主,外省游客以周边地区居多。游客出游距离以短程为主。旅游业向着多元化和融合创新的全域旅游发展,而地学旅游资源产品单一化对于大众游客缺乏吸引力,以地学旅游为核心的旅游形式和内容需要再进一步开发。通过昂普分析,提出了具体的地学旅游资源开发对策与措施,旅游产业融合产业创新,提高公园旅游一体化服务水平,打造地质与人文一体旅游,发展以世界级地质公园地学旅游为主的多元化旅游活动和旅游产品,打造有效的地学旅游宣传推广体系。公园作为地学和文化综合旅游目的地,应加强区域间旅游合作建设,拓宽公园旅游市场。 相似文献
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